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ChemInform Abstract: A Concise Total Synthesis of (.+-.)-cis- and (.+-.)-trans-Clavicipitic Acids by Combinatorial Use of Directed Lithiation and Fluoride Ion- Induced Elimination-Addition Reaction of 1-(Triisopropylsilyl)gramine Derivatives.

✍ Scribed by M. IWAO; F. ISHIBASHI


Publisher
John Wiley and Sons
Year
2010
Weight
33 KB
Volume
28
Category
Article
ISSN
0931-7597

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✦ Synopsis


A Concise Total Synthesis of (±)-cis-and (±)-trans-Clavicipitic Acids by Combinatorial Use of Directed Lithiation and Fluoride Ion-Induced Elimination-Addition Reaction of 1-(Triisopropylsilyl)gramine Derivatives.

-The key steps in the synthesis of the title compounds (VIII) and (IX) are regioselective lithiation of the gramine (I) and formation of the diester (VI).