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Chemically Modified β-Cyclodextrins as Supramolecular Carriers in the Biphasic Palladium-Catalyzed Cleavage of Allylic Carbonates: Activity Enhancement and Substrate-Selective Catalysis

✍ Scribed by Thibaut Lacroix; Hervé Bricout; Sébastien Tilloy; Eric Monflier


Publisher
John Wiley and Sons
Year
1999
Tongue
English
Weight
349 KB
Volume
1999
Category
Article
ISSN
1434-193X

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✦ Synopsis


Catalytic amounts of chemically modified β-cyclodextrins modified cyclodextrins. The process of molecular recognition between the cyclodextrin and the substrate allowed us to allowed us to achieve, in high yields, the deprotection of various water-insoluble allylic carbonates in a genuine two-perform substrate-selective catalytic reactions which cannot be achieved in homogeneous or biphasic media with phase system without co-solvent. The catalytic activities were up to 300 times higher than those observed without conventional transition metal catalysts.

usually prevents the quantitative recovery of the catalytic