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Chemical synthesis at solid interfaces. On the use of conducting polythiophenes equipped of adequate linkers allowing a facile and highly selective cathodic SN bond scission with a fully regenerating resin process

✍ Scribed by J.F. Pilard; G. Marchand; J. Simonet


Publisher
Elsevier Science
Year
1998
Tongue
French
Weight
684 KB
Volume
54
Category
Article
ISSN
0040-4020

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✦ Synopsis


Electrogenerated polythiophenes were evaluated as Merrifield-like resins for the anchoring of amine functions together with deprotection processes. Suitable linkers were terminated with a fully regenerable aromatic sulfonamide moiety. The S-N bond was cleaved to liberate the amine with high selectivity under very mild conditions by cathodic means with amine liberation. Moreover a facile recycling process of the resin allows the further grafting of various amine functions.