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Charge-transfer interactions of excited molecules with inorganic anions: the role of spin-orbit coupling in controlling net electron transfer

✍ Scribed by A. Treinin; I. Loeff; J.K. Hurley; H. Linschitz


Publisher
Elsevier Science
Year
1983
Tongue
English
Weight
583 KB
Volume
95
Category
Article
ISSN
0009-2614

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✦ Synopsis


Radical yields in simple anion-organic triplet charge-transfer interactions are interpreted in terms of spin-orbit coupliig in an incipient product radical, as evidenced by increasing yield with increasing I,?F] in cases where k> radicals with zero orbital momentum are formed_ Nitrite may also quench by energy rrzmsfer. The interactions of electronically excited molecules with inorganic anions in polar solvents have been studied extensively [l--4], with special interest being focused recently on the possibility of using such systems as redox couples for solar energy storage, e.g. the anthraquinone-Cl-