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Caracterisation d'oxydes catalyseurs a base de cuivre et de chrome par diffraction X, spectroscopie infra-rouge et reflectance diffuse

✍ Scribed by G. Wrobel; J. Arsene; M. Lenglet; A. D'Huysser; J.P. Bonnelle


Book ID
103906573
Publisher
Elsevier Science
Year
1981
Weight
479 KB
Volume
6
Category
Article
ISSN
0390-6035

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✦ Synopsis


A cubic phase close to that of 3'Cr203 has been observed in copper chromite catalysts with atomic ratio 0,8 ~< Cu/Cr ~< 1,5. The infra-red spectroscopy shows that Cr 6÷ ions should be necessary for the stability of the phase.

Cr 3+ ions in tetrahedral environment have been observed in all the catalysts by diffuse reflectance spectroscopy. In reduced state, cubic structure is kept, with formation of Cu metal. The phase is now stabilised by hydroxyls and inversion decreases.