✦ LIBER ✦

Biomimetic Total Synthesis of (±)-Pallavicinolide A

✍ Scribed by Jia-Qiang Dong; Henry N. C. Wong

Publisher: John Wiley and Sons
Year: 2009
Tongue: English
Weight: 394 KB
Volume: 121
Category: Article
ISSN: 0044-8249
DOI: 10.1002/ange.200806335

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✦ Synopsis

Abstract

Vom Teil zum Ganzen: Die erste Totalsynthese des natürlich vorkommenden Diterpens Pallavicinolid A ist gelungen. Besonders hervorzuheben sind drei biomimetische Umwandlungen: eine basenunterstützte Grob‐Fragmentierung, eine Singulettsauerstoff‐Oxidation und eine intramolekulare Diels‐Alder‐Cycloaddition.magnified image

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