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Bioinspired Molecular Design of Light-Harvesting Multiporphyrin Arrays.

✍ Scribed by Myung-Seok Choi; Tomoko Yamazaki; Iwao Yamazaki; Takuzo Aida

Publisher
John Wiley and Sons
Year
2004
Weight
69 KB
Volume
35
Category
Article
ISSN
0931-7597

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✦ Synopsis

Abstract

For Abstract see ChemInform Abstract in Full Text.

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Ο€-Electronic conjugation is not necessary to facilitate long-range energy migration and transfer: A rapid (k =1.04Γ—10 s ) and efficient (Ξ¦ =71 %) energy transfer from the 28 photoexcited zinc porphyrin units to the focal free-base porphyrin unit occurs in a large, star-shaped dendritic multiporphyri