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Belousov–Zhabotinskii type oscillations with amino acids or peptides as organic substrates in the presence of Mn2+ and Fe(phen)32+ as coupled catalysts

✍ Scribed by Hexing Li; Ronghua Jin


Publisher
John Wiley and Sons
Year
1998
Tongue
English
Weight
126 KB
Volume
30
Category
Article
ISSN
0538-8066

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✦ Synopsis


Nine amino acids, aspartic acid, glycine, serine, tyrosine, alanine, glutamic acid, threonine, cystine, phenylalanine, and two peptides, and two peptides, glycine-glycine peptide, glutamic acid-cystine-glycine peptide, give rise to damped oscillations of the Belousov-Zhabotinskii(BZ) type in a batch reactor. Both and are essential for most of 2ϩ 2ϩ

Mn Fe(phen) 3 those oscillations; and the oscillations in and are also observed. The role 3ϩ 3ϩ

[Mn ] [Fe(phen) ] 3 of two metallic ions played in the oscillations are analyzed, showing that catalyzes the 2ϩ Mn oxidation of the amino acids or peptides by to produce some intermediates which Ϫ BrO 3 effectively reduce Br 2 to Br Ϫ catalyzed by