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Assignment and Power Series Analysis of the FIR Fourier Transform Spectrum of Cyanamide Using a Multimolecule Ritz Program

✍ Scribed by Giovanni Moruzzi; Wolfgang Jabs; B.P. Winnewisser; Manfred Winnewisser


Publisher
Elsevier Science
Year
1998
Tongue
English
Weight
303 KB
Volume
190
Category
Article
ISSN
0022-2852

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✦ Synopsis


The "Ritz" program, originally written for the analysis of the Fourier transform spectra of the methanol isotopomers and presented in previous papers, has been extended in order to analyze the spectra of other molecules. This program evaluates the term values involved in the assigned transitions by the Rydberg-Ritz combination principle, and can tackle such perturbations as Fermi-type resonances or Coriolis interactions. As a first application of the extended version, we present an investigation of the Fourier transform spectrum of cyanamide between 25 and 980 cm-1. More than 16 000 lines have been assigned. Our Ritz database now comprises a list of more than 19 000 assigned lines (including of the microwave and FIR lines available in the JPL database) and more than 3900 term values. All of the lines presented in this paper correspond to transitions within the ground and first excited inversion levels of the ground vibrational state of the small-amplitude modes. Copyright 1998 Academic Press.