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Artificial neural networks as a multivariate calibration tool: modeling the FeCrNi system in x-ray fluorescence spectroscopy

✍ Scribed by A. Bos; M. Bos; W.E. van der Linden


Publisher
Elsevier Science
Year
1993
Tongue
English
Weight
657 KB
Volume
277
Category
Article
ISSN
0003-2670

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✦ Synopsis


The performance of artificial neural networks (ANNs) for modeling the Cr-Ni-Fe system in quantitative x-ray fluorescence spectroscopy was compared with the classical Rasberry-Heimich model and a previously published method applying the linear learning machine in combination with singular value decomposition. Apart from determining lf ANNs were capable of modeling the desired non-linear relationships, also the effects of using non-ideal and noisy data were studied. For this goal, more than a hundred steel samples with large variations in composition were measured at their primary and secondary K, and KS lines. The optimal calibration parameters for the Rasberry-Heinrich model were found from this dataset by use of a genetic algorithm. ANNs were found to be robust and to perform generally better than the other two methods in calibrating over large ranges.