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Application of the MPB theory to the analysis of the ion-free layer thickness

โœ Scribed by R. Andreu; M. Molero; J.J. Calvente; C.W. Outhwaite; L.B. Bhuiyan

Publisher
Elsevier Science
Year
1996
Tongue
English
Weight
563 KB
Volume
41
Category
Article
ISSN
0013-4686

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โœฆ Synopsis

The concept of ion-free layer thickness is examined on the basis of contemporary theories of the electrical double layer. A comparison between surface excesses derived from Modified Poisson-Boltzmann fMPB and URMPBl and mean field tGC and UDCA) theories is oerformed. The influence of unequal distances of closest approach for cations and anions in the analysis of experimental surface excesses is cancelled to a significant extent by inclusion of self-atmosphere and exclusion volume effects. An application is made to the mercury/aqueous LiCI, NaCl and KC1 interfaces.

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