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Anharmonicity effects on the vibrational predissociation of the NeI2(B 3Πu+, ν) complex: A close-coupling infinite-order sudden treatment

✍ Scribed by O. Roncero; J. Campos-Martínez; A.M. Cortina; P. Villarreal; G. Delgado-Barrio


Publisher
Elsevier Science
Year
1988
Tongue
English
Weight
410 KB
Volume
148
Category
Article
ISSN
0009-2614

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✦ Synopsis


A model previously applied to study the vibrational predissociation (VP) of He-I?(B, v) is extended to treat the VP of Ne-l2 (B, v) in the region of initial vibrational excitation 28 4 US 34. Due to the anhannonicity of the diatomic subunit, the usually predominant channel for VP, Au= -1, becomes energetically forbidden. This gives rise to oscillations of the VP rate as a function of u that no longer follows the typical superlinear behaviour shown in the low diatomic excitation regime.