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Analysis of polyethylene wear debris using micro-Raman spectroscopy: A report on the presence of beta-carotene

✍ Scribed by Hahn, David W. ;Wolfarth, Debra L. ;Parks, Nancy L.


Publisher
John Wiley and Sons
Year
1997
Tongue
English
Weight
83 KB
Volume
35
Category
Article
ISSN
0021-9304

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✦ Synopsis


This paper describes micro-Raman spectroscopy of ultrahigh molecular weight polyethylene wear debris isolated from revised knee replacements. The novel application of micro-Raman spectroscopy to the analysis of in vivogenerated wear debris was used to evaluate the chemical nature of individual, retrieved polyethylene particles. The analysis revealed the presence of ␤-carotene on particles from both synovial fluid and tissue samples. Raman analysis of retrieved polyethylene tibial inserts also revealed localized ␤-carotene signals within the primary wear region. In this paper, a mechanism is suggested that may account for the coupling of ␤-carotene and polyethylene wear debris. We also discuss the origin of ␤-carotene within the implanted joint and the implications that ␤-carotene, an antioxidant, has for the overall host response to polyethylene orthopedic components.