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An efficient procedure to evaluate long-range coulombic interactions within the framework of the LCAO–CO method for infinite polymers

✍ Scribed by Lucjan Piela; Joseph Delhalle


Publisher
John Wiley and Sons
Year
1978
Tongue
English
Weight
602 KB
Volume
13
Category
Article
ISSN
0020-7608

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✦ Synopsis


Abstract

A very efficient and exact method for calculating the long‐range effects in polymers is reported. The method is based on the multipole expansion within the Fock operator, and exact summation up to infinity is carried out. Only a small number of oneelectron integrals have to be considered, while in the traditional approach one has to compute a large number of twoelectron integrals. Results on LiH model polymer have been obtained with a remarkable accuracy within a negligible computing time.