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An efficient method for the calculation of generalized overlap amplitudes for core photoelectron shake-up spectra

✍ Scribed by Hans Ågren; Hans Jørgen Aa. Jensen


Publisher
Elsevier Science
Year
1987
Tongue
English
Weight
492 KB
Volume
137
Category
Article
ISSN
0009-2614

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✦ Synopsis


Using a Gelfand-Tsetlin N-electron basis and a graphical unitary group approach, an efficient method is derived for the calculation of generalized overlap amplitudes of the form Xj,"' = (Y""'(N-l)lrE,,l%r'Y'o'(N)),where Y""(N-l)and!r'fO'(N)denote complete active space wavefunctions and p is a core orbital index. Using this method the computational effort to obtain #,"I is negligible compared to the wavefunction optimization.