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An ab initio study on the mechanism of the ketene-imine cycloaddition reaction

✍ Scribed by Sordo, J. A.; Gonzalez, Javier; Sordo, T. L.

Book ID
125452729
Publisher
American Chemical Society
Year
1992
Tongue
English
Weight
891 KB
Volume
114
Category
Article
ISSN
0002-7863

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The cycloaddition reaction of FCH=C =O and NH,CH=NH leading to 2-azetidinone was studied theoretically at the level of R H F / ~-~~G and R H F / ~-~~G \* . Two possible mechanisms via a gauche or trans intermediate were compared. The obtained results show that the reaction proceeds in a gauche mann