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Alkylating agents from sugars: Synthesis of chlorambucil derivatives carried by chiral glycosyl glycerols derived from D-Glucosamine

✍ Scribed by Fernando Iglesias-Guerra; José I. Candela; Eugenia Blanco; Felipe Alcudia; José M. Vega-Pérez


Book ID
102071829
Publisher
John Wiley and Sons
Year
2002
Tongue
English
Weight
97 KB
Volume
14
Category
Article
ISSN
0899-0042

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✦ Synopsis


Abstract

Chlorambucilamide derivatives involving chiral glycosyl glycerols derived from D‐glucosamine were synthesized in good yield by coupling the chlorambucil moiety to the amino group of ω‐amino‐(ω‐1)‐hydroxyalkyl 2‐acylamino‐4,6‐O‐benzylidene‐2‐deoxy‐β‐D‐glucopyranosides, and subsequent hydrolysis of the benzylidene group. The starting material was easily available from 2‐acetamido‐2‐deoxy‐D‐glucose. The bonding of 2,3,4,6‐tetra‐O‐pivaloyl‐β‐D‐galactopyranosylamine to chlorambucil by formation of an amide function is also described. Chirality Chirality 14:199–203, 2002. © 2002 Wiley‐Liss, Inc.