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Alkaloid catalyzed asymmetric synthesis III the addition of mercaptans to 2-cyclohexene-1-one; determination of enantiomeric excess using 13C NMR.

✍ Scribed by R. Helder; R. Arends; W. Bolt; H. Hiemstra; Hans Wynberg


Publisher
Elsevier Science
Year
1977
Tongue
French
Weight
117 KB
Volume
18
Category
Article
ISSN
0040-4039

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✦ Synopsis


The addition of mercaptans to a,B-unsaturated systems is an important reaction in biosynthetic processes2 as well as in synthesis.3 We wish to report the formation in excellent yields of a series of B-ketosulfides in enantiomeric excess up to 50% by the addition of mercaptans to 2-cyclohexene-l-one in the presence of catalytic quantities of quinine.4 R--SH