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Adiabatic approach to non-radiative transitions: Exact transition rates of order Δ2

✍ Scribed by V. Denner; M. Wagner

Book ID
103372560
Publisher
Elsevier Science
Year
1983
Tongue
English
Weight
273 KB
Volume
46
Category
Article
ISSN
0038-1098

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📜 SIMILAR VOLUMES

Non-radiative transitions: Fundamental d
Non-radiative transitions: Fundamental difficulties of the adiabatic base approach
✍ M. Wagner 📂 Article 📅 1983 🏛 John Wiley and Sons 🌐 English ⚖ 552 KB

## Abstract The adiabatic base approach is extensively used in literature (“Condon” approximation, “non‐Condon” approximations). Two fundamental difficulties are indicated: (a) for large Huang‐Rhys factors it is not the non‐adiabaticity operator which governs the non‐radiative decay but tunneling;

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A self-organized chemical system is described by a set of rate equations for a primary and a partial system. The partial system acts as an internal driving force to regulate the primary system. Thermal equilibrium of the primary system is broken by coupling with the partial system and there is a cha