Non-adiabatic effects in third-harmonic
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André D. Bandrauk; Nadia Gélinas
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Article
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1986
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Elsevier Science
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English
⚖ 424 KB
A coupled-equations approach is used to calculate four-photon transition amplitudes in a third-harmonic generation process for the Cl1 molecule. It is shown that non-adiabatic interactions between Rydberg and valence states interfere with radiative interactions at high intensities (I> lo8 W/cm'), th