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Ab initio studies of chemical equilibria. Equilibria containing first row hydrides AH2, AH3, and AH4 and their positive ions

✍ Scribed by Vladimir Kellö; Miroslav Urban; Petr Čársky; Zdeněk Slanina


Publisher
Elsevier Science
Year
1978
Tongue
English
Weight
383 KB
Volume
53
Category
Article
ISSN
0009-2614

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✦ Synopsis


Equilibrium constants were calculated for fourteen simple reactions involving AH*, AH3, and A_% fust row hydrides and their positive ions_ Except for the "experimental" correlation energies used, the theoretical approach is entirely nonempki-Cal in character. The results suggest that if the correlation effects were accounted for k a more sophisticated way, most of the c&dated equilibrium constants would be more reliible than the available experimental data_