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Ab initio calculation of deuteron quadrupole coupling constants for low-lying rovibrational levels of HD in its X 1Σg+ and B 1Σu+ states

✍ Scribed by J. Vojtík; I. Paidarová; V. Špirko; J. Šavrda; M. Petráš


Publisher
Elsevier Science
Year
1989
Tongue
English
Weight
483 KB
Volume
157
Category
Article
ISSN
0009-2614

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✦ Synopsis


Deuteron quadrupole coupling constants of rovibrational levels of HD in its X 'xl and B '1: states have been calculated from molecular wavefunctions which explicirly describe vibrational motion. The quadrupole coupling constants obtained exhibit significant vibrational and rotational dependence. A marked difference between the X 'x2 and B 'Z: quadrupole hyperfine patterns is predicted. Some aspects for the future theoretical interpretation of the hyperfine structure of laser-induced fluorescence and infrared saturated absorption spectra of diatomic molecules are outlined.