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A Two-Dimensional Experiment That Separates Decoupling Sidebands from the Main Peaks

✍ Scribed by Eriks Kupc̆e; Ray Freeman


Publisher
Elsevier Science
Year
2001
Tongue
English
Weight
61 KB
Volume
151
Category
Article
ISSN
1090-7807

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✦ Synopsis


Broadband decoupling techniques generate undesirable cycling sidebands. The new two-dimensional technique described here allows separation of these sidebands from the main peaks by spreading the sideband responses in the indirectly detected dimension (F(1)) according to their frequency separations from the parent peaks, leaving the main resonances at zero frequency in F(1). This trace at zero frequency shows a thousandfold suppression of the residual sidebands, making possible the detection of very weak signals from dilute constituents of the sample. The experimental results can be displayed as one-dimensional "quiet decoupling" spectra without any significant loss of sensitivity. The new technique (DESIRE-decoupling sideband resolved spectroscopy) is simple, robust, and straightforward to implement.