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A phosphorus–tin cage molecule with an extremely shielded 31P nucleus: P4[Sn(C6H5)2]3

✍ Scribed by Gernot Heckmann; Herbert Binder; Dirk Bongert


Publisher
John Wiley and Sons
Year
1998
Tongue
English
Weight
199 KB
Volume
36
Category
Article
ISSN
0749-1581

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✦ Synopsis


The structure of the compound was deduced from the 119Sn and 31P NMR spectra

3 and it was shown to be a structural analogue of the hetero-nortricyclene

The apical phosphorus atom P 4 S 3 . exhibits an extremely negative 31P chemical shift of [554.65 ppm, and the basal phosphorus atoms also resonate at high Ðeld strengths. The 31P spectrum includes all tin satellite signals of the [mono-117@119Sn] isotopomers. The spectra are analyzed as spin systems (A, M \ 31P ; X \ 117@119Sn). The 31P data for analogous tricyclic A 2 A@MX cage molecules are presented and discussed.