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A novel synthesis of linear polyenes via conjugate addition of cuprates to α,β-γ,δ-diunsaturated sulfones followed by SO2 extrusion

✍ Scribed by Ferdinand Näf; René Decorzant; Sina D. Escher


Book ID
104219578
Publisher
Elsevier Science
Year
1982
Tongue
French
Weight
193 KB
Volume
23
Category
Article
ISSN
0040-4039

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✦ Synopsis


The two 1,3-butadienyl Z-propenyl sulfones 5 and 6, 1,3,5-heptatrlene synthons,have been transformed into the trl-and tetraenes 1 -4 by alkylcuprate addltlon and Ramberg-Backlund

SO2 extrusion

The reaction stereochemistry 1s discussed

The undecatrlenes 1 and 2, isolated from Galbanum"L, also occur, together with the undeca tetraenes 2 and 4, In the seaweeds ~z~~opterzs pZagzogrmu