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A Novel Strategy to Incorporate Carbon Nanotubes into Thermoplastic Matrices

✍ Scribed by Petra Pötschke; Sven Pegel; Michael Claes; Daniel Bonduel


Publisher
John Wiley and Sons
Year
2007
Tongue
English
Weight
400 KB
Volume
29
Category
Article
ISSN
1022-1336

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✦ Synopsis


Abstract

Multiwalled carbon nanotubes (MWNT) are introduced into thermoplastic matrices (polycarbonate and polyamide) by melt blending using polyethylene (PE) based concentrates with high MWNT loadings (24–44 wt.‐%). MWNT surfaces were treated with a metallocene‐based complex to afford the in‐situ polymerization of ethylene directly from the surface. The resulting concentrates showed excellent MWNT pre‐dispersion. Due to the high interfacial energy between MWNT and PE, the nanotubes migrate into matrix polymers with lower interfacial energies, like polycarbonate and polyamide, and thereby remain in their excellent dispersion state. Thus, electrical percolation is achieved at lower MWNT contents as compared to direct incorporation. For polycarbonate it is shifted from 0.75 to 0.25 wt.‐%.

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