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A novel o-quinodimethane strategy for an active metabolite of vitamin D3. A total synthesis of 25-hydroxy Windaus-Grundmann ketone

✍ Scribed by Hideo Nemoto; Masahiro Ando; Keiichiro Fukumoto


Publisher
Elsevier Science
Year
1990
Tongue
French
Weight
231 KB
Volume
31
Category
Article
ISSN
0040-4039

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✦ Synopsis


A highly diastereoselective total synthesis of 25-hydroxy Windaus-Grundmann ketone (2) was achieved via a novel regiocontrolled C-C bond formation by an intramolecular epoxide ring opening reaction of the bissulfonyl epoxide (19) as a key step, which was derived stereoselectively by the thermolysis of