A Nonadiabatic Theory for Ultrafast Catalytic Electron Transfer: A Model for the Photosynthetic Reaction Center
β Scribed by Serge Aubry; Georgios Kopidakis
- Publisher
- Springer Netherlands
- Year
- 2005
- Tongue
- English
- Weight
- 914 KB
- Volume
- 31
- Category
- Article
- ISSN
- 0092-0606
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π SIMILAR VOLUMES
In order to elucidate the role of special pair chlorophyll in photosynthetic
Rigorous quantum dynamics simulations have been performed to test the path-integral centroid formulation proposed by Voth, Chandler and Miller for quanta1 rate constants in a simple class of models for electron transfer reactions in the tight-binding limit. Fully dynamical quantum Monte Carlo simul
The rate expression for the superexchange reaction in a three-component system, involving a donor, a bridging intermediate and a distant acceptor, is derived using the spin-boson model for the primary electron transfer in a photosynthetic reaction center. In this model, a vector spin for SU( 3) grou