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A new two-phase route to cadmium sulfide quantum dots using amphiphilic hyperbranched polymers as unimolecular nanoreactors

✍ Scribed by Yunfeng Shi; Jiamiao Liang; Lanbo Liu; Lin He; Chunlai Tu; Xinqiu Guo; Bangshang Zhu; Chengyu Jin; Deyue Yan; Tao Han; Xinyuan Zhu


Publisher
John Wiley and Sons
Year
2010
Tongue
English
Weight
689 KB
Volume
120
Category
Article
ISSN
0021-8995

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✦ Synopsis


Abstract

A new two‐phase route was developed to prepare monodisperse cadmium sulfide (CdS) quantum dots (QDs) with a narrow size distribution. In a two‐phase system, chloroform and water were used as separate solvents for palmitoyl chloride functionalized hyperbranched polyamidoamine (HPAMAM‐PC) and cadmium acetate/sodium sulfide, respectively. The amphiphilic HPAMAM‐PC, with a hydrophilic dendritic core and hydrophobic arms, formed stable unimolecular micelles in chloroform and was used to encapsulate aqueous Cd^2+^ ions. After the reaction with S^2−^ ions from the aqueous phase, monodisperse and uniform‐sized CdS QDs stabilized by HPAMAM‐PC unimolecular micelles were obtained. © 2010 Wiley Periodicals, Inc. J Appl Polym Sci 120:991–997, 2011