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A new synthesis of allylic alcohols or their derivatives via reductive elimination from γ-phenylthio-β-nitroalcohols with tributyltinhydride

✍ Scribed by Noboru Ono; Akio Kamimura; Aritsune Kaji


Publisher
Elsevier Science
Year
1984
Tongue
French
Weight
210 KB
Volume
25
Category
Article
ISSN
0040-4039

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✦ Synopsis


Allylic alcohols are readily prepared by the Bu3SnH-promoted elimination reaction from y-phenylthio-8-nitroalcohls which are obtained by the joint reaction of nitroolefins, thiophenol, and aldehydes.

In this paper we wish to report a new synthetic method of allylic alcohols or their derivatives (4_) starting from cr-nitro olefins (1). Our new method consists of two key steps, namely, one step-introduction of phenylthio and hydroxyalkyl groups into l_ by the joint reaction of three components (1,