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A new semi-empirical method of correcting large-scale configuration interaction calculations for incomplete dynamic correlation of electrons

✍ Scribed by Franklin B. Brown; Donald G. Truhlar


Publisher
Elsevier Science
Year
1985
Tongue
English
Weight
639 KB
Volume
117
Category
Article
ISSN
0009-2614

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✦ Synopsis


We show thar large-basis-se1 confiigurallon inleraction calculations includmg al1 single and double excltahons from n wmplctc-active-space optimized by MC SCF melhods recover an approlumatcly wnstant ktction of Ihe ealemal wrreladon energy. Therefore. by scakng this conlribution to the energy, more accurate potential energy NI-WS, barrier helghu to chemical reactions, and porential energy surraces can be calculated.