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A new look at fluorescence depolarization and the dynamics of anisotropic rotational diffusion

✍ Scribed by K. Razi Naqvi

Publisher: Elsevier Science
Year: 1987
Tongue: English
Weight: 563 KB
Volume: 136
Category: Article
ISSN: 0009-2614
DOI: 10.1016/0009-2614(87)80276-2

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✦ Synopsis

Existing derivations of the time-dependent fluorescence anisotropy of an asymmetric molecule constitute a straightforward application of Favro's work on the rotational diffusion equation (RDE), and make no contribution to the elucidation of rotational dynamics as such. A new approach is developed, and the problem formulated in the parlance of conventional reaction kinetics by demonstrating, with the aid of the method of moments, that the RDE is completely equivalent to a set of ordinary linear differential equations, formally identical with those used to describe a first-order series-parallel reaction scheme.

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