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A hypothesis for conformational restriction in complexes of formyl compounds with boron Lewis acids. Experimental evidence for formyl CH--O and CH--F hydrogen bonds

✍ Scribed by E.J Corey; Jeffrey J Rohde; Axel Fischer; Mihai D Azimioara


Book ID
104255998
Publisher
Elsevier Science
Year
1997
Tongue
French
Weight
189 KB
Volume
38
Category
Article
ISSN
0040-4039

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✦ Synopsis


The X-ray crystal structures of the complexes C6H5CHOoBF31 and H2C=C(CH3)CHO.BF32 reveal that the BF3 is coordinated to the oxygen lone pair which is syn to the formyl proton and, further, that the formyl proton and one B-F bond are in plane (eclipsed) with respect to the C-O-B triad, as shown in 1. A preference