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A General Approach to Aza-Heterocycles by Means of Domino Sequences Driven by Hydroformylation

✍ Scribed by Etienne Airiau; Thomas Spangenberg; Nicolas Girard; Angèle Schoenfelder; Jessica Salvadori; Maurizio Taddei; André Mann

Book ID: 102796746
Publisher: John Wiley and Sons
Year: 2008
Tongue: English
Weight: 796 KB
Volume: 14
Category: Article
ISSN: 0947-6539
DOI: 10.1002/chem.200801795

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✦ Synopsis

Abstract

The development of hydroformylative domino reactions of easily accessible vinyl acetamides is described. Extremely regioselective hydroformylation of terminal double bounds provides a transient N‐acyliminium that can be trapped by various nucleophiles to give several aza‐heterocylic scaffolds in a diastereoselective manner.

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