✦ LIBER ✦

A fluidised-bed membrane reactor for the catalytic partial oxidation of methane to synthesis gas

✍ Scribed by L. Mleczko; T. Ostrowski; T. Wurzel

Publisher: Elsevier Science
Year: 1996
Tongue: English
Weight: 509 KB
Volume: 51
Category: Article
ISSN: 0009-2509
DOI: 10.1016/0009-2509(96)00218-7

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✦ Synopsis

A fluidised-bed membrane reactor was proposed as reaction engineering meam for performing the catalytic partial oxidation of methane to synthesm gas (syngas) in a safe and stable nuumer, and to achieve high syng~ yields at elevated pressures and low temperatures. In ocder to analyse the potential of this reactor design a reaction engineering model was developed. Simulation studies performed with this model for palladium and ceramic membranes indicated that in the fluidi~d-bed membrane reactor higher syngas yields can be achieved compared to the fluidised bed. Furthermore, under certain conditions the integrated product separation allowed to overcome the thermodynamic constraints. Syng~ yield in the fluidhu~-bed membrane reactor strongly ~ on the permeation rate and the selectivity of the separation. For the ceramio membrane the interaction between membrane and bed hydrodynamics was found to be of primary im~ce; in order to achieve high syngas yields the separation unit should contact mainly with the emulsion phase.

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