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A combined XPS-UPS-EELS study of nitrogen adsorbed on clean and barium-promoted iron surfaces: The nature of the precursor to dissociation

✍ Scribed by C.N.R. Rao; G.Ranga Rao; K. Ppabhakaran


Publisher
Elsevier Science
Year
1987
Tongue
English
Weight
287 KB
Volume
134
Category
Article
ISSN
0009-2614

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✦ Synopsis


For Nz on a clean Fe surface, the adsorbed precursor in a parallel orientation becomes predominant around 110 K, while at lower temperatures it coexists with a weakly adsorbed species. On a Ba-promoted Fe surface, however, N2 is present exclusively in the precursor state in the temperature range 80-l 50 K following moderate exposure. Besides exhibiting a low N-N stretching frequency of 1530 cm-', the precursor shows a clear separation between the 50 and lx levels in the UPS; the precursor dissociates to give a nitridic species around 160 K.

* Contribution No. 389 from the Solid State and Structural

Chemistry Unit.