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A CNDO insight to the alcoholysis of N-sulphinylamines in ethanol, using copper(II) chloride as catalyst

✍ Scribed by W.K. Glass; I.J. King; A. Shiels


Publisher
Elsevier Science
Year
1977
Tongue
English
Weight
192 KB
Volume
25
Category
Article
ISSN
0020-1693

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✦ Synopsis


Using the CNDO/2 method, the electron densities in p-NOz, p-Cl, and p-H N-Sulphinylanilines were computed. The electron densities at sulphur were found to be proportional to the Hammett a-values of the substituents and also to log k, for the alcoholysis. The activation energy, Arrhenius factor and AS' values for the system copper(H) chloride, ethanol and N-sulphinylaniline are reported.