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A classical trajectory study of the angular momentum coupling model the influence of anisotropic polarizability on the lifetimes of complexes formed in ion—molecule collisions

✍ Scribed by F.J. Schelling; A.W. Castleman Jr.


Publisher
Elsevier Science
Year
1984
Tongue
English
Weight
695 KB
Volume
111
Category
Article
ISSN
0009-2614

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✦ Synopsis


The influence of the anisotropic polarizabilities of the neutral molecule on the lifetimes of complexes formed in ionmolecule collisions of Na+ with N2 and CO* were determined using a classical trajectory calculation. Lifetimes are found to be increased substantiaIIy over those calculated for the same systems having isotropic polarbzabilities The fmdings lend further support to the angular momentum coupling model of Ferguson and co-workers proposed to account for factors influencing the vibrational relaxation of ions.