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4-(N,N-Dimethylamino)benzonitrile solvated by a polar molecule: Structural demand for charge-transfer state formation

✍ Scribed by T. Kobayashi; M. Futakami; O. Kajimoto


Book ID
103026394
Publisher
Elsevier Science
Year
1986
Tongue
English
Weight
372 KB
Volume
130
Category
Article
ISSN
0009-2614

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✦ Synopsis


Van der Waals complexes consisting of 4-( N-N-dimethylamino)benzonitrile and a polar molecule such as Hz0 and CFsH were produced in a free jet. The laser-induced fluorescence spectra of their O-O bands showed blue-shifts in contrast to the van der Waals complexes with rare-gas atoms. Their emission spectra did not contain any charge-transfer component which is known to be easily observed in a polar solvent. These facts are interpreted in terms of the structure of the van der Waals complexes.