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1H NMR Study of the Conformation of Metallapentacycles N—C—C—O—M [M = Rh(III) and Ir(III)] Resulting in a Karplus-Type Relationship for Vicinal H–C(sp3)–N(sp13)–H Coupling Constants

✍ Scribed by M. Luisa Jimeno; José Elguero; Daniel Carmona; M. Pilar Lamata; Emilio San José


Publisher
John Wiley and Sons
Year
1996
Tongue
English
Weight
318 KB
Volume
34
Category
Article
ISSN
0749-1581

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✦ Synopsis


The complete analysis of the 'H NMR spectra of [ (C,Me,)lr(glycinate)CI] and [ (C,Me,)Ir(N-methyl-g1ycinate)Clj provide information for the conformational analysis of the five-membered N-C-C-0-Ir ring.

A Karplus relationship has been established for these metallacycles [ 3J(H,H) = 8.9 cos' 4 -1.0 cos 4 + 0.81.