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195Pt-NMR Spectroscopy of Catalytically Active Complexes. Extremely Large Spin-Spin Coupling between Platinum and Tin

✍ Scribed by Dr. Karl-H. A. Ostoja Starzewski; Dr. Paul S. Pregosin


Book ID
101551317
Publisher
John Wiley and Sons
Year
1980
Tongue
English
Weight
237 KB
Volume
19
Category
Article
ISSN
0044-8249

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✦ Synopsis


An extremely high coupling constant of 28954 Hz (^1^J(^195^Pt^119^Sn))—the highest one‐bond spin‐spin coupling yet found—has been measured for [PtCl(SnCl~3~)(PEt~3~)~2~]. In combination with SnCl~2~, platinum‐phosphane complexes are excellent homogeneous catalysts for hydrogenation and hydroformylation reactions. ^195^Pt‐NMR spectroscopy is extremely sensitive to changes of the coordination sphere and is therefore well suited to the study of such catalysts.