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13C T1 NMR study of arylmercury compounds. Barriers to rotation about the carbon–mercury bond

✍ Scribed by Ruthanne D. Thomas; Keith E. Rowland


Publisher
John Wiley and Sons
Year
1988
Tongue
English
Weight
486 KB
Volume
26
Category
Article
ISSN
0749-1581

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✦ Synopsis


Barriers to rotation about the preferred axis, C-4-Hg-C-4, were determined for diphenyl-, bis(o-toly1)-and bis(m-toly1)-mercury from 13C T , relaxation times as a function of temperature in DMSO and in 1,1,2,2-tetrachloroethane-CCt,. Based on results for the unsymmetrical compound phenyl(o-tolyl)mercury, the rotation about the preferred axis is interpreted as rotation about the carbon-mercury bond. The average barrier to internal rotation of 3.6 0.6 kcal mol-' is constant as a function of both methyl substitution and coordinating and non-coordinating solvents.