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1,2,3-Tricarbonylverbindungen, VIII. Die Verwendung von Fluorenylidentriphenylphosphoranen in der Carbonyl-Olefinierung nachWittig. Versuche mit 1,2,3-Indantrion, 1,2,3-Trioxo-2,3-dihydrophenalen, Glyoxal und Terephthalaldehyd

✍ Scribed by Schönberg, Alexander ;Singer, Erich ;Schulze-Pannier, Heidemarie


Publisher
Wiley (John Wiley & Sons)
Year
1973
Tongue
English
Weight
492 KB
Volume
106
Category
Article
ISSN
0009-2940

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✦ Synopsis


The Use of Fluorenylidenetriphenylphosphoranes in Witrig Olefin Synthesis. Experiments with 1 ,2,3-Indanetrione, 1,2,3-Trioxo-2,3-dihydrophenalene, Glyoxal, and Terephthalaldehyde

The fluorenylidenetriphenylphosphoranes 1 and 2 react with the cyclic 1,2,3-tricarbonyl compounds 5 and 6 to yield the corresponding ethylene5 9-12 and triphenylphosphine oxide. Treatment of 1 and 2 with glyoxal or terephthalaldehydc affords the dienes 20-23.25 was obtained by reaction of 9-phenanthrenecarbaldehyde with 1.

Statements found in t h e literature concerning the rcactrvity of 1 are discussed.